Description of the thesis topic

erosols and clouds are key players in tropospheric chemistry. These tiny particles suspended in the air, with a radius ranging from a few nanometres to tens of micrometres, impact atmospheric composition, represent one of the largest uncertainties in climatic projections and cause millions of deaths worldwide every year. Hence, they have enormous societal and economic consequences. Nonetheless, there is still a knowledge gap preventing us from describing the chemical evolution of aerosols and clouds during their atmospheric lifetime.
Water molecules in bulk liquid are stable and inert under ambient conditions. In sharp contrast, it was very recently shown that the local orientation of water molecules at an air/water interface induces an electric field that generates spontaneous radicals in micron-sized droplets. This production does not involve any catalysts such as light or heat. It is an intrinsic property of the air/water interface, and therefore potentially ubiquitous in the troposphere.
This PhD project aims to unravel the atmospheric importance of this interfacial chemistry by means of (i) laboratory-based investigations, (ii) field observations and (iii) modelling. These activities will take place in the frame of an ERC founded project.

Work Context

The recruited person(s) will perform either laboratory-based experiments, field measurements or numerical modelling, depending in the applicant's profile.
The experimental activities will involve various advanced high-resolution mass spectrometers (Orbitrap, Vocus, …), optical techniques (fluorescence, optical tweezers,…), aerosol flow tubes and an atmospheric simulation chamber.
The modelling aspects will cover the development of a new aerosol chemistry module for box models up to meso-scale modelling.

The position is located in a sector under the protection of scientific and technical potential (PPST), and therefore requires, in accordance with the regulations, that your arrival is authorized by the competent authority of the MESR.

Constraints and risks

n/a

Additional Information

This research is conducted in the frame of the ERC SOFA